70's and 90's. 80's was too full of trendy bs (much like 00's) without much substance. I might have to give 90's an edge because of the availible technology, they were able to push the envelope a but further (Jurassic Park, Independence Day, Matrix) even if the movies that employed them weren't the greatest.
Some other 90's movies not mentioned
Schindler's List
Shawshank Redemption
Pulp Fiction
Good Fellas
Se7en
Silence of the Lambs
Although, I think the 40's is regarded as having the most "best of all time" movies
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